Enrichment of alkanes within a phytoplankton bloom during an in situ iron enrichment experiment in the western subarctic Pacific     

Sohiko Kameyama  Urumu Tsunogai  Fumiko Nakagawa  Motoki Sasakawa  Daisuke D. Komatsu  Akira Ijiri  Junko Yamaguchi  Takeo Horiguchi  Hiroshi Kawamura  Aika Yamaguchi  Atsushi Tsuda 《Marine Chemistry》2009,115(1-2):92-101

During the Subarctic Pacific Iron Experiment for Ecosystem Dynamics Study ΙΙ (SEEDS-II), we monitored variations in the concentrations of non-methane hydrocarbons (NMHCs), CH₃Cl, N₂O, and CH₄ within a phytoplankton bloom. Stable isotopic compositions were also determined to evaluate the sources of the variations. Although there was little variation in either the concentrations or the stable isotopic compositions of alkenes, CH₃Cl, N₂O, and CH₄ during the 23-day observation period, alkane concentrations increased substantially as the phytoplankton bloomed. The column-integrated quantities of alkanes increased to 3 times pre-bloom levels for C₂H₆, 5 times for C₃H₈, and 20 times for n-C₄H₁₀. The δ¹³C values of both C₂H₆ and C₃H₈ remained almost constant while concentrations increased, whereas that of n-C₄H₁₀ increased by about 12‰. To evaluate the sources of the alkanes produced during the bloom, we compared their δ¹³C values with those of alkanes produced in axenic phytoplankton cultures in our laboratory. We concluded that during the SEEDS-ΙΙ experiment the major portions of C₂H₆ and C₃H₈ were produced during the autolysis of diatoms cells, whereas n-C₄H₁₀ was produced during autolysis of other phytoplankton cells such as cryptophytes and dinoflagellates.  相似文献   

Are measurements from excised leaves suitable for modeling diurnal patterns of gas exchange of intact leaves?     

Yoshiyuki Miyazawa  Makiko Tateishi  Hikaru Komatsu  Tomo'omi Kumagai  Kyoichi Otsuki 《水文研究》2011,25(18):2924-2930

To examine the feasibility of using ecophysiological data from excised leaves for a meteorological simulation model of gas exchange, we compared the obtained gas exchange rates and the modelled ones using excised leaves and those using intact leaves. Instantaneous gas exchange rates of excised leaves and stomatal control in response to environmental conditions were not significantly different from those of attached leaves. Modelled gas exchange rates based on excised leaf data showed a good fit to the diurnal patterns of in situ measurements. This suggests that use of excised leaf data to predict gas exchange of intact leaves is permissible as long as the effects of excision are pre‐screened as described in this paper. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

Magnetometer survey of the proposed Sirente meteorite crater field,central Italy: Evidence for uplifted crater rims and buried meteorites     

Jens ORM   David Gomez‐Ortiz  Patrick C. McGuire  Herbert Henkel  Goro Komatsu  Angelo Pio Rossi 《Meteoritics & planetary science》2007,42(2):211-222

Abstract— The Sirente crater field consists of a 120 m wide, rimmed main depression flanked to the northwest by about 30 smaller depressions. It has been dated to the first centuries A.D. An impact origin is suggested, but not confirmed. The small size combined with the properties of the target material (carbonate mud) would neither allow shock features diagnostic of impact, nor projectile vaporization. Consequently, a meteoritic component in the sediments would be very localized. At impacts of this size the projectile most likely is an iron meteorite. Any iron meteorites on the ground surface would, in Iron Age Europe, have been removed shortly after the event. However, if the depressions are of impact origin they should contain meteorites at great depth in analogy with known craters. The magnetic properties of iron meteorites differ distinctly from the very low magnetic sediments and sedimentary rocks of the Sirente area. We have used a proton precession magnetometer/gradiometer to produce magnetic anomaly maps over four of the smaller depressions (～8 m diameter), as well as two crossing profiles over a fifth depression (～22 m diameter). All show distinct magnetic anomalies of about 20 nT, the larger depression up to 100 nT. Magnetic modeling shows a best fit for structures with upturned strata below their rims, excluding a karstic origin but supporting an explosive formation. The 100 nT anomaly can only be explained by highly‐magnetic objects at a few meters depth. All together, the magnetic data provides a strong indication for an impact origin of the crater field.  相似文献   

Angular power spectrum of gamma-ray sources for GLAST: blazars and clusters of galaxies     

Shin'ichiro Ando  Eiichiro Komatsu  Takuro Narumoto  Tomonori Totani 《Monthly notices of the Royal Astronomical Society》2007,376(4):1635-1647

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Estimation of vertical profiles of leaf drying times after daytime rainfall within a Bornean tropical rainforest     

Tomonori Kume  Odair J Manfroi  Masakazu Suzuki  Katsunori Tanaka  Koichiro Kuraji  Michiko Nakagawa  Hikaru Komatsu  Tomo'omi Kumagai 《水文研究》2008,22(18):3689-3696

South‐east Asian Bornean tropical rainforests have large and complex canopy structures. To clarify how forest structure affects wet‐canopy evaporation, it is necessary to consider wet‐canopy evaporation processes within the forest canopy, such as vertical profiles of canopy drying time. In a previous study a method was proposed that utilizes sap flow measurements to estimate canopy drying time after rainfall (CDTobs) during daytime. In this present study, the method was applied to estimations of the vertical variations in CDTobs in 11 individual trees of various heights, ranging from 2·7 m to 53 m. The study derived vertical profiles and showed that the lengths of CDTobs in lower canopy trees were 2–4 h longer than those in the upper canopy trees. The new method for CDTobs profiles presented in this study, which is available for validation of multi‐layer biosphere‐atmospheric models, is a useful illustration for clarifying wet‐canopy evaporation processes in tropical rainforests. Copyright © 2008 John Wiley & Sons, Ltd.  相似文献   

Hydrogen isotopes in volcanic plumes: Tracers for remote temperature sensing of fumaroles     

Urumu Tsunogai  Kanae Kamimura  Saya Anzai  Fumiko Nakagawa  Daisuke D. Komatsu 《Geochimica et cosmochimica acta》2011,75(16):4531-4546

In high-temperature volcanic fumaroles (>400 °C), the isotopic composition of molecular hydrogen (H₂) reaches equilibrium with that of the fumarolic H₂O. In this study, we used this hydrogen isotope exchange equilibrium of fumarolic H₂ as a tracer for the remote temperature at volcanic fumaroles. In this remote sensing, we deduced the hydrogen isotopic composition (δD value) of fumarolic H₂ from those in the volcanic plume. To ascertain that we can estimate the δD value of fumarolic H₂ from those in a volcanic plume, we estimated the values in three fumaroles with outlet temperatures of 630 °C (Tarumae), 203 °C (Kuju), and 107 °C (E-san). For this we measured the concentration and δD value of H₂ in each volcanic plume, along with those determined directly at each fumarole. The average and maximum mixing ratios of fumarolic H₂ within a plume’s total H₂ were 97% and 99% (at Tarumae), 89% and 96% (at Kuju), and 97% and 99% (at E-san). We found a linear relationship between the depletion in the δD values of H₂, with the reciprocal of H₂ concentration. Furthermore, the estimated end-member δD value for each H₂-enriched component (−260 ± 30‰ vs. VSMOW in Tarumae, −509 ± 23‰ in Kuju, and −437 ± 14‰ in E-san) coincided well with those observed at each fumarole (−247.0 ± 0.6‰ in Tarumae, −527.7 ± 10.1‰ in Kuju, and −432.1 ± 2.5‰ in E-san). Moreover, the calculated isotopic temperatures at the fumaroles agreed to within 20 °C with the observed outlet temperature at Tarumae and Kuju. We deduced that the δD value of the fumarolic H₂ was quenched within the volcanic plume. This enabled us to remotely estimate these in the fumarole, and thus the outlet temperature of fumaroles, at least for those having the outlet temperatures more than 400 °C. By applying this methodology to the volcanic plume emitted from the Crater 1 of Mt. Naka-dake (the volcano Aso) where direct measurement on fumaroles was impractical, we estimated that the δD value of the fumarolic H₂ to be −172 ± 16‰ and the outlet temperature to be 868 ± 97 °C. The remote temperature sensing using hydrogen isotopes developed in this study is widely applicable to many volcanic systems.  相似文献   

Pressure responses of portlandite and H–D isotope effects on pressure-induced phase transitions     

Riko Iizuka  Hiroyuki Kagi  Kazuki Komatsu  Daichi Ushijima  Satoshi Nakano  Asami Sano-Furukawa  Takaya Nagai  Takehiko Yagi 《Physics and Chemistry of Minerals》2011,38(10):777-785

The pressure responses of portlandite and the isotope effect on the phase transition were investigated at room temperature from single-crystal Raman and IR spectra and from powder X-ray diffraction using diamond anvil cells under quasi-hydrostatic conditions in a helium pressure-transmitting medium. Phase transformation and subsequent peak broadening (partial amorphization) observed from the Raman and IR spectra of Ca(OH)₂ occurred at lower pressures than those of Ca(OD)₂. In contrast, no isotope effect was found on the volume and axial compressions observed from powder X-ray diffraction patterns. X-ray diffraction lines attributable to the high-pressure phase remained up to 28.5 GPa, suggesting no total amorphization in a helium pressure medium within the examined pressure region. These results suggest that the H–D isotope effect is engendered in the local environment surrounding H(D) atoms. Moreover, the ratio of sample-to-methanol–ethanol pressure medium (i.e., packing density) in the sample chamber had a significant effect on the increase in the half widths of the diffraction lines, even at pressures below the hydrostatic limit of the pressure medium.  相似文献   

Effects of slope gradient on runoff from bare-fallow purple soil in China under natural rainfall conditions     

Yoshitaka Komatsu  Hiroaki Kato  Bo Zhu  Tao Wang  Fan Yang  Randeep Rakwal  Yuichi Onda 《山地科学学报》2018,15(4):738-751

Purple soil is highly susceptible for overland flow and surface erosion, therefore understanding surface runoff and soil erosion processes in the purple soil region are important to mitigate flooding and erosion hazards. Slope angle is an important parameter that affects the magnitude of runoff and thus surface erosion in hilly landscapes or bare land area. However, the effect of slope on runoff generation remains unclear in many different soils including Chinese purple soil. The aim of this study was to investigate the relationship between different slope gradients and surface runoff for bare-fallow purple soil, using 5 m × 1.5 m experimental plots under natural rainfall conditions. Four experimental plots(10°, 16°, 20° and 26°) were established in theYanting Agro-ecological Experimental Station of Chinese Academy of Science in central Sichuan Basin. The plot was equipped with water storage tank to monitor water level change. Field monitoring from July 1 to October 31, 2012 observed 42 rainfall events which produced surface runoff from the experimental plots. These water level changes were converted to runoff. The representative eight rainfall events were selected for further analysis, the relationship between slope and runoff coefficient were determined using ANOVA, F-test, and z-score analysis. The results indicated a strong correlation between rainfall and runoff in cumulative amount basis. The mean value of the measured runoff coefficient for four experimental plots was around 0.1. However, no statistically significant relationship was found between slope and runoff coefficient. We reviewed the relationship between slope and runoff in many previous studiesand calculated z-score to compare with our experimental results. The results of z-score analysis indicated that both positive and negative effects of slope on runoff coefficient were obtained, however a moderate gradient(16°-20° in this study) could be a threshold of runoff generation for many different soils including the Chinese purple soil.  相似文献   

Formation mechanism of the Weddell Sea Polynya and the impact on the global abyssal ocean     

Mikitoshi Hirabara  Hiroyuki Tsujino  Hideyuki Nakano  Goro Yamanaka 《Journal of Oceanography》2012,68(5):771-796

An experiment using a global ocean–ice model with an interannual forcing data set was conducted to understand the variability in the Southern Ocean. A winter-persisting polynya in the Weddell Sea (the Weddell Polynya, WP) was simulated. The process of WP breaking out after no-WP years was explored using the successive WPs found in the late 1950s. The results suggested that the anomalously warm deep water, saline surface layer, and a cyclonic wind stress over the Maud polynya region in early winter are essential for the surface layer to be dense enough to trigger deep convections which maintain a winter-persisting polynya; also, the reanalyzed surface air temperature (SAT) over the observed polynya region is too high for an ocean–ice model’s bulk formula to yield sufficient upward heat fluxes to induce WP formation. Therefore the Weddell Polynya, a series of WPs observed from satellite in the mid-1970s, is reproduced by replacing the SAT with a climatological one. Subsequent to the successive WP events, density anomalies excited in the Weddell Sea propagate northward in the Atlantic deep basins. The Antarctic Circumpolar Current (ACC) is enhanced through the increased meridional density gradient. The enhanced ACC and its meandering over the abyssal ridges excite buoyancy anomalies near the bottom at the southwestern end of the South Pacific basin. The buoyancy signals propagate northward and eventually arrive in the northern North Pacific.  相似文献   

Mass-to-light ratio of Lyα emitters: implications of Lyα surveys at redshifts z= 5.7, 6.5, 7 and 8.8     

Elizabeth R. Fernandez  Eiichiro Komatsu 《Monthly notices of the Royal Astronomical Society》2008,384(4):1363-1376

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